Investigation of slowing down and charge-exchange of nickel and uranium ions in gases and solids in the energy range (60 - 200) MeV/u
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In this thesis new slowing down and charge-state measurements will be presented in the energy range of (60 - 200) MeV/u. These measurements were done using the Fragment Separator (FRS) facility at GSI in Darmstadt. The presented data were taken during two experimental runs. The experiments were divided into two parts. In the first part a 200 MeV/u Ni27+ beam was used. The evolution of charge states as a function of the target thickness was investigated covering both the non-equilibrium and equilibrium region. This was done with various mono-atomic materials (Z2 = 6, 7, 10, 13, 18, 22) and compound materials (ethylene, polyethylene and polypropylene). From the measured charge-state distributions the one-electron ionization and capture cross sections have been extracted. A 40 % gas-solid difference is observed in the ionization cross sections forthe mono-atomic materials. In the compound materials a 30 % difference is observed between ethylene and the polymers. The experimental cross sections for the mono-atomic materials have been compared with theoretical calculations [1, 2]. The theoretical ionization cross sections agree quitewell with the corresponding experimental ionization cross sections. In the gaseous targets the agreement between experiment and theory is better than 3 %. For the capture cross sections the agreement between experiment and theory is also very good for the lighter target materials (Z2 <= 7). For the heavier targets large deviations up to one order of magnitude are observed. These deviations are due to the increasing importance of the non-radiative capture channel in heavier target materials which is quite difficult to calculate accurately. The results motivate for further refinement of the theory in this energy region. In the second part 3 different uranium beams were used with initial energies of 61 MeV/u (U86+ incident), 85 MeV/u (U73+ incoming) and 200 MeV/u (U81+ incident) to measure the evolution of the charge states again and the energy loss as a function of the target thickness in the same materials as used in the first part plus some additional mono-atomic materials Z2 = 29, 36, 47, 54. From the measured charge-state distributionsand energy losses the mean charges and stopping forces have been extracted.At 61 MeV/u we observe a gas-solid difference in the mean charge of up to 4 charge states for the mono-atomic materials. The corresponding stopping powers (forces) at the same specific energy only show a gas-solid difference for light materials (Z2 <= 7). The stopping forces are compared with calculations done with the PASS code [3, 4], ATIMA code [5] and the Hubert et al. tables [6]. The agreement is quite good between experiment and theory. The PASS code predicts by using the experimental mean charges a gas-solid difference in the stopping force for the heavier target materials. In the data at 200 MeV/u there is a gas-solid difference in the ionization rate for U81+ ions similar to the Ni27+ results.Verknüpfung zu Publikationen oder weiteren Datensätzen
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Nuclear Instruments and Methods in Physics Research B, 245 (2006), S. 32-35